Alpha Spectrometry is a fascinating technique because it allows you to have accurate information about the radioactive decay of heavy nuclei and about the physics of the interaction of charged particles with matter. But this is a rather difficult technique, even more difficult than gamma spectrometry. The difficulties of this technique lie in the type of detector, usually a solid state silicon detector (rather expensive) that produces a very weak signal which requires, to be analyzed, very low noise amplifiers. The measurement has to be made in vacuum conditions (however not high vacuum) so that the alpha particles are not shielded from the air. The sources that are measured have to be carefully prepared so as to have a layer as thin and uniform as possible so that alpha particles are not diffused and absorbed within the source itself.
Despite these difficulties it is possible, with a fair amount of work and patience, prepare a DIY instrument that can give a lot of satisfaction.
Introduction
The alpha radioactive nuclei (typically heavy nuclei) can decay by emitting alpha particles (helium nuclei) with energies of the order of a few MeV, with spectra with lines, corresponding to the energy levels of involved nuclei . In the figure aside it is an example of energy spectrum of alpha emissions of U-238. The alpha-active nuclei are heavy nuclei with atomic number greater than 82 (lead). Examples are Polonium, Radium, Thorium, Uranium, etc …
The alpha decay has been explained theoretically by G. Gamow in the first half of the previous centurymaking use of the tunnel effect in quantum mechanics. In the figure is a graph which shows the wave function of the alpha particle inside the nucleus and outside, beyond the Coulomb barrier. Although the alpha particle does not have enough energy to overcome the barrier it is seen as outside the nucleus the wave function is not zero and thus there is a non-zero probability that the alpha particle is ejected from the nucleus. Using this model it is possible to explain with good accuracy the characteristics of alpha decay.
Solid State Detector
In a semiconductor, the equivalent of the ionization energy is the band-gap energy to promote an electron from the valence to the conduction band. In Si at room temperature, Eg = 1.1 eV, compared to ~15 eV to ionize a gas. A charged particle moving through Si therefore creates more ionization and a larger signal. When n-type and p-type silicon are put in contact, creating a p-n junction, the flow of the two different free charges across the boundary creates a depletion zone, an electrically neutral area near the junction where an internal electric field sweeps out any free charge. By reverse biasing the junction, the depletion zone can be made large, ~hundreds of microns. If an energetic charged particle ranges out in the depletion zone, an amount of ionization proportional to the particle’s initial energy will be created there, and swept out. By plating metallic ohmic contacts on the outer surfaces of the crystal, it is possible to both apply the bias and collect the free charge from the depletion zone, so that the whole assembly is a high gain, solid state version of the capacitive ionization chamber.
In our project we have used the detector shown in the image aside (thanks to Professor John Bland). It features the following technical data :
– Canberra PIPS SPD-100-12 (partially depleted) – Active area = 100mm2 – FWHM 12KeV at 5MeV – Bias Voltage = 40V – Thickness = 100μm
Signal Processing
The signal produced by the detector has very low amplitude and therefore it requires an appropriate amplification. Given the very low level of the signal you must use very low noise amplifiers, also the bias voltage must be free of ripple, which is why we have adopted a power-based batteries. The preamplifier of the signal is based on a charge sensitive preamplifier type (CSP): the current pulse generated by the detector is converted into a voltage pulse by means of the charge of a capacitor. In the scheme below it is presented ta basic diagram of a charge preamplifier :
Response of a CSP
At time domains lasting up to a few microseconds, the CSP output is the time integral of the current pulse from the PIPS/Surface barrier detector. The output rise time is approximately equal to the duration of the current pulse, although the speed of the CSP sets a lower limit to this rise time. Because the CSP Produces an output voltage step that is proportional to the time integral of the current input and remembering that :
the CSP output is proportional to the total charge (Q) from the PIPS detector. At much longer time domains the response of a CSP to a fast current pulse from a PIPS detectors is in the form of a tail pulse. A tail pulse has a fast initial rise time followed by a very long exponential decay back to the baseline. A tail pulse response from a CSP module is shown below.